Simović joined Napredak Kruševac from BSK Batajnica in 1986, making three appearances in the 1986–87 Yugoslav Second League.
[2] He would earn a transfer to Proleter Zrenjanin in 1991,[3] making 24 appearances and scoring seven goals in the final season of the Yugoslav First League.
[4] In 1993, Simović moved abroad to play for French club Brest,[5] netting three goals in the Championnat National 1 during the 1993–94 season.
He switched to Kavala in January 1996 and helped the club win promotion to the top flight that year, contributing with seven goals.
[7] After spending one more season with Kavala,[8] Simović joined fellow Alpha Ethniki club Ethnikos Piraeus in 1997.