[4] She debuted as a playback singer with the song "He Jeevan Sundar Aahe" in the Marathi film Chaukat Raja (1991), composed by Anand Modak and written by Sudhir Moghe, alongside Asha Bhosle and Ravindra Sathe.

[2] Anjali sang two iconic songs in the film, "Nagpanchamicha San Bai" and "Bhui Bhegalali Khol," with lyrics by Namdeo Dhondo Mahanor and music by Anand Modak.

She also recorded "Jeevan Tyanna Kalale Ho" with her mother Anuradha and singer Ravindra Sathe, written by Balkrishna Bhagwant Borkar and composed by Saleel Kulkarni.

Anjali's talents extended beyond films, as she recorded title tracks for TV serials like Jhoothe Sachhe Gudde Bacche (Hindi) and Olakh Sanga Na (Marathi).

Anjali has participated in numerous stage shows, including Smrutyayatra at the World Marathi Conference in Mumbai, Safarnama in Nagpur (2019),[5] and Shukratara in Pune (2023).