He was selected by the Baltimore Ravens in the fifth round of the 2010 NFL draft and won Super Bowl XLVII with them.

[citation needed] As a senior, he had 64 tackles, six sacks, and one fumble recovery to help lead Union–Endicott to a Section IV championship.

[4] In a 34–14 win over Miami (Ohio), Jones sacked their quarterback, Daniel Raudabaugh, for a loss of seven yards.

[5] On November 11, 2006, in a game at Raymond James Stadium home of the South Florida Bulls, Jones recovered the first fumble of his collegiate career.

[8] In the beginning of the second half against South Florida on November 11, Jones injured his ankle on a chop block.

[9] On November 17, Jones was held out of the game against Connecticut and according to coach Greg Robinson the decision came because, "Arthur has been too good of a football player for us to risk putting him out there and really getting him hurt.

Following Syracuse's upset win over Notre Dame he was named Big East Defensive Player of the Week and was also awarded an ESPN Helmet Sticker for his performance.

[2] In 2009, Jones missed three games, playing in nine and made 19 tackles (7 for losses) and 1.5 sacks and recovered 2 fumbles and was named First-team All-Big East for the second consecutive season.

The Ravens advanced to Super Bowl XLVII for the second time in franchise history against the San Francisco 49ers.

[23] After returning from his suspension, Jones started all eight games he appeared in and tallied 30 tackles before being placed on injured reserve on December 19, 2016, with a groin injury.

[32] His youngest brother, Chandler, was an edge rusher for the Las Vegas Raiders who previously played for the Arizona Cardinals and New England Patriots.