At this time she was part of a circle of modern artists centred on Hampstead, London, and was one of the founders of the art movement Unit One.
At the beginning of the Second World War Hepworth and Nicholson moved to St Ives, Cornwall, where she would remain for the rest of her life.
Best known as a sculptor, Hepworth also produced drawings – including a series of sketches of operating rooms following the hospitalisation of her daughter in 1944 – and lithographs.
In 1933, Hepworth travelled with Nicholson to France, where they visited the studios of Jean Arp, Pablo Picasso, and Constantin Brâncuși.
[11] In 1933, Hepworth co-founded the Unit One art movement with Nicholson and Paul Nash, the critic Herbert Read, and the architect Wells Coates.
"[14] Hepworth married Nicholson on 17 November 1938 at Hampstead Register Office in north London, following his divorce from his wife Winifred.
On 8 February 1949, Hepworth and Nicholson co-founded the Penwith Society of Arts at the Castle Inn; 19 artists were founding members, including Peter Lanyon and Bernard Leach.
[17] Hepworth often used her garden in St Ives, which she designed with her friend the composer Priaulx Rainier, to view her large-scale bronzes.
[17] Her eldest son Paul was killed on 13 February 1953 in a plane crash while serving with the Royal Air Force in Thailand.
[27] When Hepworth returned to St Ives from Greece in August 1954 she found that Gardiner had sent her a large shipment of Nigerian guarea hardwood.
[27] Between 1954 and 1956 Hepworth sculpted six pieces out of guarea wood, many of which were inspired by her trip to Greece, such as Corinthos (1954) and Curved Form (Delphi) (1955).
Initially she hoped to follow Henry Moore's successful sale of artwork via Curt Valentin of Bucholz Gallery in New York.
[29] Hepworth's difficulties in establishing a stable gallery relationship in the United States have been attributed to many factors, including the artist's own diffidence regarding personal promotion of her work.
When Martha Jackson failed to arrange the solo American exhibition of sculptures and drawings that Hepworth demanded, Hepworth moved, in 1957, to Galerie Chalette, run by Arthur and Madeleine Lejwa, known for their close relationship with Jean Arp, and dedication to close relationships with their artists.
"[29] Three years later, having secured the Dag Hammarskjöld Memorial Commission (Single Form, 1964), she left both Chalette and Gimpel Fils, her long-time home agent, for the larger Marlborough Fine Art and Marlborough-Gerson.
[32] Hepworth greatly increased her studio space in 1960 when she purchased the Palais de Danse, a former cinema and dance hall, that was situated across the street from Trewyn.
[33] She also experimented with lithography in her late career, and produced two lithographic suites with the Curwen Gallery and its director Stanley Jones, one in 1969 and one in 1971.
To complete the large-scale piece Hepworth hired her first assistants, Terry Frost, Denis Mitchell, and John Wells.
[42] One of the editions of six of her 1964 bronze sculpture, Rock Form (Porthcurno), was removed from the Mander Centre in Wolverhampton in the spring of 2014 by its owners, the Royal Bank of Scotland and Dalancey Estates.
[43]: 95 The same year, she was inducted into Gorsedh Kernow with the bardic name Gravyor (meaning "Sculptor")[44] – this was described as an "extraordinary honour" given that she was not a Cornish native.
[46] Following her death, her studio and home in St Ives became the Barbara Hepworth Museum, which came under control of the Tate in 1980.
The first large London show since 1968, it included her well-known major abstract carvings and bronzes, as well as previously unseen photographs and a 1930s self-photogram.