She coordinated the vocals on the New Seekers' single "I'd Like To Teach The World To Sing" and was the voice behind the 1960s TV adventure series The Saint.

She also rearranged "At the Sign of the Swingin' Cymbal", an instrumental composition that served as the theme tune for Alan Freeman's Pick of the Pops.

She also founded her own group, the Barbara Moore Singers, performing alongside Glen Campbell (1970), Bobbie Gentry (1970-71) and Mike Yarwood (1972) on BBC television programmes, as well as on the soundtrack of the film The Ruling Class (1971).

The BBC, in April 1970, asked her to update Brian Fahey's "At the Sign of the Swingin' Cymbal" for Alan Freema's Pick of the Pops show.

[1] She also arranged the vocals for "I'd Like to Teach the World to Sing", a Coca-Cola commercial song from 1971 that became a hit for the New Seekers in a modified version.

After she had composed the theme for Terry Wogan's BBC Radio show, she gained a job at de Wolfe, the library music company.

She vocalised on recordings, including the Roger Webb Sound's Vocal Patterns and Moonshade albums, and scored music for commercials across Europe.

[4][3][5] She also provided the soundtrack to Anthony Stern's experimental film Serendipity in 1972, playing piano alongside musician colleagues Chris Spedding, Ray Warleigh and John Marshall.