In 1886 the congregation sold the Columbia Street building to Congregation Ahavath Acheim Anshe Ungarn and moved into the Gothic Revival-style synagogue at 172 Norfolk Street that is now the Angel Orensanz Center, the oldest surviving synagogue building in New York and the fourth-oldest in the United States.

[3] In 1906–07 the congregation built and moved into a "monumental" building on 116th Street, in the newly fashionable neighborhood of Harlem.

Costly structural damage necessitated the building's demolition, which occurred slowly throughout late 2009 and early 2010.

The current synagogue building at 118 West 95th Street (constructed in 1926) is noted for its Moorish Revival architecture.

[5] Early in the 21st century, the congregation became known for attracting large numbers of Orthodox Jewish singles to its services and programs.