Angulo made his first-team — and La Liga — debut on 23 March 2003, coming on as a late substitute in a 2–1 away loss against RC Celta de Vigo.
[4] On 30 December 2004, after appearing in only three league matches with the main squad, Angulo was loaned to Segunda División's Gimnàstic de Tarragona until the end of the season.
[6] On 25 July 2006, Angulo moved abroad for the first time in his career, joining French Championnat National club AS Cannes in a season-long loan deal.
[10] In his second season at the Andalusians he contributed nine goals in only 19 league matches, being the team's top scorer;[11] highlights included a hat-trick in a 6–2 home rout of Jerez Industrial CF on 10 January 2010.
[15] He joined Real Unión hours later,[16] scoring a career-best 13 goals in 2012–13, being team top scorer and being linked to a number of clubs also in the third division.
[19] Angulo switched clubs and countries again on 14 September 2014, joining Football League (Greece)'s Apollon Smyrnis FC.