He began working in paint and ceramic before expanding his focus to include metal and concrete reliefs.

Over the next 20 years, he created more than 100 works in Quebec and abroad, and associated with major art figures such as Salvador Dalí.

In 1967, Jordi Bonet created The Inuit Family, a rotunda that represents life in northern Newfoundland and Labrador, the work is located inside the main entrance of the Charles S. Curtis Memorial Hospital, Saint Anthony, Canada.

[citation needed] Among his other major works are the relief L’homme devant la science on the west facade of the Pavillon Adrien-Pouliot of Université Laval in Quebec, 'Citius, Altius, Fortius in the Montreal Metro station Pie-IX;[citation needed] Hommage à Gaudí, a cycle of wall sculptures in Place des Arts in Montreal; the Halifax Explosion Memorial Sculpture; and a set of stained-glass windows and sculptures in Our Lady of the Skies Chapel[4] at John F. Kennedy International Airport in New York City.

He was particularly interested in sacred works, creating artworks and liturgical objects for churches and convents in Quebec, Ontario, and elsewhere.