The Sinatra–Jobim Sessions is a 1979 double LP compilation album of American singer Frank Sinatra's work with Antônio Carlos Jobim.

The album was published only in Brazil by producer Roberto Quartin, and had never been re-released on vinyl or CD until 2010 when it was re-mastered and released under The Frank Sinatra Collection and became available worldwide.

The first two of these tracks later appeared on the 1977 UK compilation album Portrait of Sinatra, but were also included on Sinatra-Jobim Sessions, making it eagerly sought by collectors.

"Off Key (Desafinado)" was not included here and remained largely unavailable until Sinatra's The Complete Reprise Studio Recordings was released in 1995.

Sinatra and Jobim worked together for a final time in 1994 on Duets II, recording a cover of "Fly Me to the Moon".