The church was designed in 1923 by Lewiston architects Gibbs & Pulsifer, and is an imposing example of neo-Gothic architecture for a relatively small community.

The former St. Cyril and St. Methodius Church is located in the village of Lisbon Falls, at the southeast corner of Main Street (Maine State Route 125) and High Street.

The front facade is flanked by squat square towers with buttress-style projecting pilasters at the corners.

Atop the large arch is a wagon-wheel rose window, and the gable above is crested by a cross.

Alienated from other well-established cultural groups, they formed their own Catholic organization, and raised funds to build this church, which was completed in 1923.