[2] He was well known for his portrayal of the chess grandmaster Kronsteen in the James Bond film From Russia with Love (1963), a role for which he had been personally recommended by his friend Sean Connery, and as Otto Leipzig in Smiley's People (1982).

[3][4] He also had notable recurring roles as Dr. Douglas Jackson in Gerry Anderson's UFO, Captain Ferreira in the NBC miniseries Shōgun and as Gen. Bratchenko in the 1984 version of Red Dawn.

[1] He appeared in the film Kanał (1957, credited as Władysław Sheybal), directed by Andrzej Wajda, before departing for Paris and then Vienna in 1958 owing to his political opposition to the Communist Party.

[9] His other films include Casino Royale (1967), Doppelgänger (1969), The Last Valley, Puppet on a Chain, Innocent Bystanders, The Wind and the Lion, The Lady Vanishes (1979), Fire and Sword, and Red Dawn.

[12][13] Sheybal's final stage appearance was as Friedrich Nietzsche in the Pierre Bourgeade play The Eagle and the Serpent at London's Offstage Downstairs Theatre in 1988.