Between 1835 and 1846 he travelled much in the south of Europe, but in the latter year succeeded to the title and family estates in Somerset, Devon, Cornwall, and Northumberland.
These were greatly improved during his tenure, for he was a generous landlord and a public-spirited agriculturist, much noted for his herd of short-horned cattle.
He was a liberal patron of the fine arts, and formed at Wallington Hall a good collection of curious books and of specimens illustrative of natural history and ethnology.
He published, according to the Royal Society's catalogue, fifteen papers on scientific subjects, the majority dealing with geological topics in the north of England.
A biographer from the family notes that Walter changed his will in 1852, being impressed by his cousin's son; the young George Otto had been one of the couple's visitors and received hints of the secret will.
[5] A medallion head is introduced into the decorations of the hall at Wallington;[6] a portrait in oils, painted by an Italian artist about 1845, is at Nettlecombe, and a small watercolour (by Millais) is in the possession of the widow of Sir A. W.