Their debut album, Simple Things, was released in 2001; their song "Destiny" stayed in the top 100 of the UK Single Charts.

[2] The pair also remixed Terry Callier's "Love Theme From Spartacus" and songs by Lenny Kravitz, Sneaker Pimps and Lambchop.

In 2001, they released their debut album, Simple Things, which featured collaborations with vocalists Mozez, Sia, and Sophie Barker.

[4][5] Live appearances after the album's release consisted of Binns and Hardaker along with guest vocalists and other musicians, with as many as 20 performers on stage at once.

[6] Zero 7 released their third album, The Garden, in May 2006, which contained vocals performed by Binns as well as guest vocalists Sia and Swedish folk musician José González.

The album included contributions from jazz and soul singer Eska Mtungwazi as well as folk artist Martha Tilston.

[13] In October 2019, the duo released another single titled "Swimmers" with additional vocals courtesy of UK based singer Jem Cooke.

[17] Then on 3 April they released their first new single, "The Crowd", from forthcoming album with California west coast based artist Swim Surreal.