He pursued formal education in filmmaking, earning a Higher National Diploma (HND) in Video Production from Bournemouth University in 1999.

Zamani has directed over 300 music videos for prominent artists, including Snoop Dogg, Enrique Iglesias, T-Pain, Lil Wayne, French Montana, Drake, and P. Diddy Zamani expanded into commercial directing, working with major brands such as Luxor Casino Hotel, LG, Black Mask Rum, and H2 Rose.

The film, starring William McNamara and Kaylynn Kubeldis, tells the story of a grieving cardiologist who finds new purpose after meeting a blind girl.

Due to its commercial success, a sequel, Angels Fallen: Warriors of Peace, was released, featuring Cuba Gooding Jr., Denise Richards, and Randy Couture.

The sequel became a #1 hit on Amazon Prime's Top 10 list in the U.S.[9][10] Ali Zamani received two Silver Davey Awards (2012) for The Comeback Kid and Love Like Magic.