In singles, Phillips-Moore twice reached the semifinals of the Australian Championships, in 1961 and 1968.

Phillips-Moore won the 1968 ATP Auckland Open defeating Onny Parun in a five-set final.

Phillips-Moore won the 1971 ATP Stuttgart Open defeating István Gulyás in the final.

Phillips-Moore died on 29 June 2023, at the age of 85.

This biographical article relating to Australian tennis is a stub.