Founded in 2021, they play in the Venezuelan Segunda División.

[1] Initially a proposal to rename LALA FC to Bolívar SC,[2] which later did not materialize, Bolívar were founded in 2021.

They started to play in the year's Segunda División, and announced former international footballer Luis Vera as their manager.

[3] In the 2023 Segunda División, Bolívar reached the finals in both Apertura and Clausura tournament, losing the Apertura finals to Ureña but defeating Marítimo de La Guaira in the Clausura finals; in the tournament's finals, they lost to Ureña and missed out promotion.

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