After the release of her third album Freya's Love Songs (非愛不可。心林凡) in 2007, Lim went to Boston University to pursue a master's degree in Applied Communication.

In 1999, Lim's singing talent was discovered by Taiwan well-known music producer Benjamin Lin Ming Yang.

She was singing acclaimed Mandopop singer Sandy Lam's Night's Too Dark at a KTV with her friends when Benjamin Lin chanced upon her voice, and she was signed on to What's Music International Incorporated.

She was involved in the musical play Love Mileage (愛情里程) which was staged at Taiwan Huashan Arts Centre between 10 and 13 September 2009.

[3] Lim held her first ticketed solo concert 林凡 Freya&Friends 幸福零缺口犀利演唱會 at Taipei International Convention Center (TICC) on 18 August 2012.