Simms was rated as the 87th overall incoming recruit by ESNPU HoopGurlz 100 and committed to play for West Virginia.

[1] Simms played in 8 games for the Mountaineers during her freshman year and averaged 3.1 points.

[3] During her first season competing at ODU, Simms was named the Conference USA Newcomer of the Year.

[6] She also led the entire league in scoring at 22.2 points, while also finishing in 5th for overall field goal percentage at .460.

Her scoring average of 26.0 broke a ODU school record previously held by Anne Donovan since 1980–1981.

[11] Simms played in 10 career games for the Mystics in 2017, scoring a high of 4 points on June 9, 2017, against the Minnesota Lynx.

Simms re-signed with the Fever as a training camp contract for the 2018 season, but ultimately didn't make the team and was waived on May 4, 2018.

[17] She was cut just before the 2022 season opener, but was brought back on a Hardship Contract, as the Mercury were missing players due to injury and Overseas commitments.