[3] Moray recorded and released the single Sprig of Thyme in May 2004, and in the autumn appeared on the Oysterband's Big Session Volume 1 album.

On 6 July 2007, The Independent featured Sweet England in its "Cult Classic" series, affirming its impact and influence on the modern folk scene.

On 1 February 2010 it was announced that Jim Moray's fourth album In Modern History would be given away as a covermount CD with the June edition of Songlines magazine, with a street date of 30 April 2010.

Along with singer and guitarist Sam Carter, in 2014 Moray launched a new band named False Lights to play traditional music with electric instruments.

Their album Salvor, produced by Moray, was released in February 2015 and they announced headline shows at Folk East, Trowbridge Village Pump and Homegrown festivals.

Moray's sixth album Upcetera was released on September the 30th 2016, featuring orchestral arrangements blended with electric rhythm section, electronic soundscapes and, on several tracks, viol played by Damon Albarn and Nico Muhly collaborator Liam Byrne.

On Moray's seventh album The Outlander he explored a more stripped down style of playing and arranging influenced by the British folk revival of the 1960s and 70s and featuring Bellowhead fiddle player Sam Sweeney on six tracks.

In February 2023 Moray entered Abbey Road Studios to re-record songs from across his career to celebrate 21 years of recording and performing.

[6] During 2005 Moray produced and performed on James Raynard's debut album Strange Histories, released in September 2005 on One Little Indian records.

In 2008 he wrote and produced the song The Wishfulness Waltz for his sister Jackie Oates' second album The Violet Hour,[1] as well as playing all the instruments on the track.

Moray's early live shows frequently featured video projections and lighting effects, something relatively uncommon in British folk music.

In November 2013 Moray staged a 10th Anniversary Performance of his first album Sweet England at the Union Chapel in Islington, London featuring a string section and special guests including Bella Hardy, Jackie Oates, Keston Cobblers Club and Maz O'Connor.

In 2017 Moray assembled a 10-piece band featuring strings, woodwind and an electric rhythm section to play the music from his Upcetera album on tour.

[9] As an opening act or collaborator, Moray has toured with Oysterband, Eliza Carthy, Billy Bragg, Richard Thompson, Ani Di Franco, Bellowhead, The Cecil Sharp Project and John McCusker.