He was born in Göttingen, and worked as the physician-in-chief in the Greek Navy, after Prince Otto of Bavaria became King of the newly constituted Kingdom of Greece.
He collected a large corpus of folklore material (tales, folksongs, riddles, translations of the Bible and One Thousand and One Nights from his informant Vasilis Sakellaris (Βασίλης Σακελλάρης), an Arvanite Orthodox priest from Poros.
In 1855 he published a small volume of the materials he collected, under the name Noctes Pelasgicae vel Symbolae ad cognoscendos Dialectos Graeciae Pelasgicae collatae cura Dr. Caroli Henrici Theodori Reinhold.
[1][2] After Reinhold's death, some of his notes fell in the hands of Gustav Meyer, who published them in his Albanesische Studien (1883–1896).
His transcriptions and grammatical notes (463 pages) were published in Tirana, Albania (2005).