[9] Liao is now signed under A Legend Star Entertainment Corp., a company founded by former Channel [V] Taiwan director, Andy Chang.

They, then, officially signed a contract with EMI Capitol on December 2, 2006, appointing Zhuang as the leader of the newly formed group Lollipop.

[19] Four months later, on May 25, a second EP titled Summer's First Experience[21] was released along with a photobook compiled with photos taken in Okinawa, as well as a DVD.

During the summer of 2007, Liao and the other members of Lollipop made their acting debut in the drama Brown Sugar Macchiato,[23] a collaboration with Hey Girl.

[26] Liao wrote the lyrics for the opening theme of the said drama, entitled "黑糖秀"(Hei Tang Xiu).

[27] On September 26, 2007, Lollipop visited Hong Kong to promote their television soundtrack Brown Sugar Macchiato.

This was their first overseas promotional activity ever since their debut, and a huge fan turnout caused a great commotion at the shopping mall where they were having their autograph session.

[31] Gyashan entered Mandarin charts in the number one position, outselling F4's album Waiting for You – Await Your Love (在這裡等你) which was released on the same day.

[43] During this period, Liao also guest starred in The Legend of Brown Sugar Chivalries, as well as writing lyrics for two songs in this drama, including the opening theme, Cang Jing Ge (藏經閣).

[47] The V-Power concert united Liao, Zhuang, and Liu with other Black Angle Crew members for a dance performance.

[53] In 2009, Lollipop made its first lyric contributions to other artists, which are included in the mini album of the group Choc7,[54] composed of seven members selected from the same show.

On September 12, 2009, a short film in which Liao was cast as the main lead, and directed and shot by Liu A-wei called The Great Escape (廖問之越V風雲)[59] was aired on Channel [V] Taiwan.

[9] Former Lollipop members, Qiu and himself had been undergoing a series of secret training for the past year after they had separated with the band in 2009.

[62] On September 10, they had their first concert at the Hong Kong Kowloon Bay International Trade and Exhibition Center to promote their single.

[67] They signed a contract under A Legend Star Entertainment Corp., a company founded by former Channel [V] Taiwan director, Andy Chang.

[75] In addition with the theme of love, 365 album also emphasized the "Golden Triangle" concept to capture each members' individual firm and confidence and also to represent their strong brotherhood.

[73] Moreover, the track list also includes a solo song for each member,[77] and a collaboration with Kimberley Chen entitled "Internet".

[77] Besides his music career, Liao Xiao Jie has been cast on Next TV's new television series called 愛味男女 (Flavor Lover) as a main lead, Tang Ai Wei, together with Tsai Yi-chen.