As well as involved in the distribution of Religious material, and education, the Society employed itinerant preachers travelling in Ireland.
In August 1807 the society asked Thomas Charles(a Welsh Calvinistic Methodist, Dr. David Bogue (a non-conformist preacher), the Rev.
Joseph Hughes (a Baptist), and Samuel Mills (member of the British Foreign Bible Society) to visit Ireland to report on the state of Protestant religion in the country.
Their report initiated amongst other things, considerable involvement in the provision of education in Ireland in the nineteenth century.
One of the activities of the LHS was the production of educational and religious material in the Irish Language.