With help from his brother Henri (1804 – 1887), he wrote Le Véritable Manuel des conjugaisons ou la science des conjugaisons mise à la portée de tout le monde (Paris: Dépôt central des publications classiques, 1842), a reference guide to French verb conjugation, in 1842.
While the Le Véritable Manuel enjoyed considerable success, it was L'Art de conjuguer that became the staple for students of French.
It went through scores of editions under this title until the 1990s, when it was renamed Bescherelle: La conjugaison pour tous in France (it continued to be published as L'Art de conjuguer in other Francophone territories, notably Quebec).
Louis-Nicolas Bescherelle was the publisher of the National Dictionary (Dictionnaire national) or the Universal Dictionary of the French Language (Dictionnaire universel de la langue française), a major dictionary of the 19th century and L'Instruction popularisée par l'illustration (Popularized Instruction for Illustration, now as Popular Instruction for Illustration) in 1851.
He also wrote on an illustrated book on naval history of France, England and Holland (commonly today as the Netherlands) which was published in 1868.