[3] She first became interested in acting after watching Nicolas Bary's 2008 adaption of Trouble at Timpetill, based on the novel by Henry Winterfeld.

[4] Bajrami's first role was in the 2011 television film Adèle's Choice by Olivier Guignard, where she played an 8-year-old Albanian student whose family was threatened with expulsion.

[9] Bajrami was praised for her portrayal of Sophie in the 2019 independent French film Portrait of a Lady on Fire.

That same year, she played the role of Emma in Cedric Khan's Happy Birthday, which focused on a dysfunctional family reunion.

[10][11] In 2020, it was announced that Bajrami was making her directorial debut with the film The Hill Where Lionesses Roar.