[3] She appeared on Emily's Reasons Why Not opposite Heather Graham[3][4] and the Adult Swim cult hit Delocated, as well as successful appearances on Aaron Sorkin projects such as Tina Lake on Sports Night and as the First Lady's Chief of Staff, Lily Mays, on The West Wing.
Dajani has appeared in a variety of television episodes on such shows as Sex and the City ("Critical Condition")[5] and its prequel The Carrie Diaries (where she played a completely different, yet more major, role), Ugly Betty, The King of Queens, Body of Proof, Curb Your Enthusiasm, and Law & Order: Special Victims Unit, and starred in the CBS film The Lost Valentine alongside Betty White.
[3][11] Dajani is a founding member of Malaparte Theatre Company, whose artistic director was Ethan Hawke.
[12] In 1993 she appeared alongside Calista Flockhart, Ethan Hawke, Steve Zahn in an off-Broadway play, Sophistry.
[15] Dajani appears in Brady Kiernan's 2011 romantic drama film Stuck Between Stations, alongside Josh Hartnett and Michael Imperioli.