She divided her time between New York City and Boca Raton, Florida.

Her film career began with playing the sister of Judy Holliday, whom Bond resembled, in The Marrying Kind in 1952.

[6] She is best known for her 1953 Tony Award-winning performance as Fay Fromkin in the original Broadway production of Wish You Were Here.

[7] Bond's work on television included being the main dancer on Inside U.S.A. With Chevrolet, which led to her being featured in photographs about the program in an article in Life magazine.

[8] She also appeared on ABC Album, Appointment with Adventure, The Arthur Murray Party, The Colgate Comedy Hour, The Ed Sullivan Show, Four Star Revue, Frankie Laine Time, Playhouse 90, The Saturday Night Revue with Jack Carter, and The Texaco Star Theatre Starring Milton Berle.