The title track was an important early single for the group, featuring Smokey Robinson's lead voice, a chorus led by his wife Claudette and an orchestra of strings.

Other hits like "What's So Good About Goodbye" and "I've Been Good To You" are included, plus three covers of easy listening standards: "I've Got You Under My Skin" written by Cole Porter, "On the Street Where You Live" from the Broadway musical My Fair Lady, and "Speak Low" by Ogden Nash and Kurt Weill, on which both Smokey and Claudette Robinson sing lead.

I'll Try Something New also features a rare lead by Miracles baritone Ronnie White on "A Love That Can Never Be", and a lead by Claudette Robinson on "He Don't Care About Me".

This album is one of the few Miracles albums to feature the complete original six-member group lineup on its cover: Marv Tarplin, Claudette Rogers Robinson, Smokey Robinson, Bobby Rogers, Ronnie White, and Pete Moore.

I'll Try Something New and four other Miracles albums were released on CD as part of the 2009 Motown 50th Anniversary limited edition CD release The Miracles – Depend On Me: The Early Albums.