All 16 locations city-wide offer services and programs for adults, teens and children residing in London and the surrounding counties of Oxford, Middlesex, and Elgin.

This not only allowed for an economical expansion of the branch, but also offered the library a more central location in the city's downtown core.

[15] As part of this renovation, a portion of the branch's northern section was remodelled to become CBC Radio One's CBCL-FM's new broadcast studio for new local and regional programming such as London Morning and Afternoon Drive and as well as digital content.

Michael Ciccone is currently the 12th CEO of the London Public Library, succeeding Susanna Hubbard Krimmer in August 2019.

On the morning of 13 December 2023, the London Public Library was the subject of a cyberattack that resulted in a major system outage.