Wesley three years later caused Atmore's name to be inserted in the deed of declaration as one of the members of the legal conference.

In the discussions on the polity and position of Methodism which took place immediately after Wesley's death, Atmore took a leading part and contributed to the consolidation of the Wesleyan Methodist church.

His ministry until 1825 was in the following towns: York, Edinburgh, Halifax, Bristol, London, Birmingham, Manchester, Wakefield, Liverpool, Leeds, Hull, Salford, Sheffield.

He was author of the Methodist Memorial (with information on early Methodism), first published in 1801, and later re-issued; Discourses on the Lord's Prayer, 1807, also republished; and also pamphlets and occasional sermons.

Another publication called "The Whole Duty of Man" is a volume described as Devout Meditations in its 5th edition was printed and published by Nuttall, Fisher and Co, Liverpool, and written by Rev Charles Atmore.