The TOT elementary layers are not rigidly connected to each other but are separated by a free space: the interlayer hosting hydrated cations and water molecules.
Only more expandable vermiculite and some rarer alumino-silicate minerals (zeolites) with inner channel structure can exhibit a higher CEC than smectite.
Smectites are formed from the weathering of basalt, gabbro, and silica-rich volcanic glass (e.g., pumice, obsidian, rhyolite, dacite).
The highly porous (with a large and easily accessible specific surface) and very reactive volcanic ashes rapidly reacted with seawater.
In civil engineering works, it is routinely used as a thick bentonite slurry when excavating deep and narrow trenches in the ground to support the lateral walls and to avoid their collapse.
Smectites, more commonly called bentonite, are candidate as buffer and backfill materials to fill the space around high-level radioactive waste in deep geological repositories.